Atomic Layer Engineering of Aluminum-Doped Zinc Oxide Films for Efficient and Stable Perovskite Solar Cells

Simple item record

Full item record

dc.contributor.authorKruszyńska, Joanna
dc.contributor.authorOstapko, Jakub
dc.contributor.authorOzkaya, Veysel
dc.contributor.authorSurucu, Belkis
dc.contributor.authorSzawcow, Oliwia
dc.contributor.authorNikiforow, Kostiantyn
dc.contributor.authorTavakoli, Mohammad Mahdi
dc.contributor.authorYadav, Pankaj
dc.contributor.authorKot, Małgorzata
dc.contributor.organizationInstitute of Physical Chemistry Polish Academy of Sciencesen
dc.contributor.organizationCBRTP – Research and Development Center of Technology for Industry, Warsaw, Polanden
dc.contributor.organizationKaramanoglu Mehmetbey University Department of Metallurgical and Materials Engineering, Karaman, Turkeyen
dc.contributor.organizationDepartment of Electrical Engineering and Computer Science Massachusetts Institute of Technology, USAen
dc.contributor.organizationDepartment of Solar Energy School of Technology Pandit Deendayal Energy University Gandhinagar, Indiaen
dc.contributor.organizationBTU COTTBUS – SENFTENBERG, Cottbus, Germanyen
dc.contributor.organizationDepartment of Physics, Indian Institute of Technology Roorkee Roorkee, Haridwar, Indiaen
dc.date.accessioned2023-03-01T15:14:55Z
dc.date.available2023-03-01T15:14:55Z
dc.date.issued2022-05-22
dc.description.abstractAtomic layer deposition (ALD) has been considered as an efficient method to deposit high quality and uniform thin films of various electron transport materials for perovskite solar cells (PSCs). Here, the effect of deposition sequence in the ALD process of aluminum-doped zinc oxide (AZO) films on the performance and stability of PSCs is investigated. Particularly, the surface of AZO film is terminated by diethylzinc (DEZ)/H2O (AZO-1) or trimethylaluminum (TMA)/H2O pulse (AZO-2), and investigated with surface-sensitive X-ray photoelectron spectroscopy technique. It is observed that AZO-2 significantly enhances the thermal stability of the upcoming methylammonium lead iodide (MAPbI3) layer and facilitates charge transport at the interface as evidenced by photoluminescence spectroscopes and favorable interfacial band alignment. Finally, planar-type PSC with AZO-2 layer exhibits a champion power conversion efficiency of 18.09% with negligible hysteresis and retains 82% of the initial efficiency after aging for 100 h under ambient conditions (relative humidity 40 ± 5%). These results highlight the importance of atomic layer engineering for developing efficient and stable PSCs.en
dc.description.sponsorshipNational Science Centre
dc.identifier.citationAdv. Mater. Interfaces 2022, 9, 2200575. https://doi.org/10.1002/admi.202200575en
dc.identifier.doi10.1002/admi.202200575
dc.identifier.urihttps://open.icm.edu.pl/handle/123456789/22366
dc.language.isoen
dc.publisherWileyen
dc.relationSONATA BIS 10, 2020/38/E/ST5/00267en
dc.rightsUznanie autorstwa 4.0 Międzynarodowe*
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/*
dc.subjectatomic layer depositionen
dc.subjectelectron transporting layersen
dc.subjectperovskitesen
dc.subjectsolar cellsen
dc.subjectstability of perovskite solar cellsen
dc.titleAtomic Layer Engineering of Aluminum-Doped Zinc Oxide Films for Efficient and Stable Perovskite Solar Cellsen
dc.typearticleen
Files for this record
Original bundle
Now showing 1 - 2 of 2
Name: Adv Materials Inter - 2022 - Kruszy ska - Atomic Layer Engineering of Aluminum%E2%80%90Doped Zinc Oxide Films for Efficient and.pdf
Size: 3.65 MB
Format: Adobe Portable Document Format
Description: manuskrypt
Download
Name: admi202200575-sup-0001-suppmat.pdf
Size: 1.5 MB
Format: Adobe Portable Document Format
Description: supporting information
Download
License files
Name: license.txt
Size: 236 B
Format: Plain Text
Description:
Download
Belongs to collection
Artykuły ICHF PAN / IPC PAS Articles